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Nanofiltration for drinking water treatment: a review

《化学科学与工程前沿(英文)》 2022年 第16卷 第5期   页码 681-698 doi: 10.1007/s11705-021-2103-5

摘要: In recent decades, nanofiltration (NF) is considered as a promising separation technique to produce drinking water from different types of water source. In this paper, we comprehensively reviewed the progress of NF-based drinking water treatment, through summarizing the development of materials/fabrication and applications of NF membranes in various scenarios including surface water treatment, groundwater treatment, water reuse, brackish water treatment, and point of use applications. We not only summarized the removal of target major pollutants (e.g., hardness, pathogen, and natural organic matter), but also paid attention to the removal of micropollutants of major concern (e.g., disinfection byproducts, per- and polyfluoroalkyl substances, and arsenic). We highlighted that, for different applications, fit-for-purpose design is needed to improve the separation capability for target compounds of NF membranes in addition to their removal of salts. Outlook and perspectives on membrane fouling control, chlorine resistance, integrity, and selectivity are also discussed to provide potential insights for future development of high-efficiency NF membranes for stable and reliable drinking water treatment.

关键词: nanofiltration     drinking water     disinfection byproducts     micropollutants     selectivity    

Emergency drinking water treatment in source water pollution incident-technology and practice in China

Xiaojian ZHANG , Chao CHEN ,

《环境科学与工程前沿(英文)》 2009年 第3卷 第3期   页码 364-368 doi: 10.1007/s11783-009-0027-2

摘要: An investigation into emergency potable water treatment technologies was conducted to investigate China’s water pollution situation. In order to confirm optimum parameters, the technological efficiency of each pollutant was obtained. About 100 contaminants were tested to find the emergency treatment technologies, most of which were found to be positive. This paper presents the three largest and most significant water pollution incidents in China to date, analyzing cases such as the nitrobenzene pollution incident in the Songhua River in November 2005, the cadmium pollution incident in the Beijiang River in December 2005, and the water crisis with odorous tap water in Wuxi City in May 2007.

关键词: emergency drinking water treatment     water pollution     adsorption     oxidation     precipitation    

What have we known so far about microplastics in drinking water treatment? A timely review

《环境科学与工程前沿(英文)》 2022年 第16卷 第5期 doi: 10.1007/s11783-021-1492-5

摘要:

• 23 available research articles on MPs in drinking water treatment are reviewed.

关键词: Microplastics     Drinking water treatment     Coagulation     Flocculation     Membrane     Filtration    

Comparative genotoxicity of water processed by three drinking water treatment plants with different watertreatment procedures

Ting Zhang, Heze Liu, Yiyuan Zhang, Wenjun Sun, Xiuwei Ao

《环境科学与工程前沿(英文)》 2020年 第14卷 第3期 doi: 10.1007/s11783-020-1214-4

摘要: Genotoxicity of substances is unknown in the water after treatment processes. Genotoxicity decreased by activated carbon treatment but increased by chlorination. Halogenated hydrocarbons and aromatic compounds contribute to genotoxicity. Genotoxicity was assessed by umu test; acute and chronic toxicity by ECOSAR. Inconsistent results confirmed that genotoxicity cannot be assessed by ECOSAR. Advanced water treatment is commonly used to remove micropollutants such as pesticides, endocrine disrupting chemicals, and disinfection byproducts in modern drinking water treatment plants. However, little attention has been paid to the changes in the genotoxicity of substances remaining in the water following the different water treatment processes. In this study, samples were collected from three drinking water treatment plants with different treatment processes. The treated water from each process was analyzed and compared for genotoxicity and the formation of organic compounds. The genotoxicity was evaluated by an umu test, and the acute and chronic toxicity was analyzed through Ecological Structure- Activity Relationship (ECOSAR). The results of the umu test indicated that biological activated carbon reduced the genotoxicity by 38%, 77%, and 46% in the three drinking water treatment plants, respectively, while chlorination increased the genotoxicity. Gas chromatograph-mass spectrometry analysis revealed that halogenated hydrocarbons and aromatic compounds were major contributors to genotoxicity. The results of ECOSAR were not consistent with those of the umu test. Therefore, we conclude that genotoxicity cannot be determined using ECOSAR .

关键词: Drinking water     Treatment process     Genotoxicity     Umu test     Ecological Structure-Activity Relationship    

Seasonal and treatment-process variations in invertebrates in drinking water treatment plants

Zhiling Wu, Xianchun Tang, Hongbin Chen

《环境科学与工程前沿(英文)》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1354-6

摘要: Abstract • Seasonal and treatment-process variations in invertebrates in a DWTP were analyzed. • The propagation and leakage of invertebrates in BAC filter were the most serious. • Invertebrates can survive and reproduce in chlorine disinfected clear water tanks. • Proportions of endogenous invertebrates increased along the treatment process. Problems associated with excessive propagation and leakage of invertebrates in drinking water have received increasing attention in recent years. We performed a monthly survey of invertebrate abundance and taxa in the effluent of each treatment stage in a drinking water treatment plant between May 2015 and April 2016 and analyzed seasonal and treatment-process variations in invertebrates. The results showed that invertebrate abundances in raw water, effluent of the biological activated carbon (BAC) filter, and finished water significantly correlated with water temperature, whereas no correlation was observed between water temperature and invertebrate abundance in the effluents of the sedimentation tank and sand filter. The dominant taxa in the effluent of each treatment stage were rotifers, nematodes, and crustaceans. The sedimentation tank could efficiently remove invertebrates with an annual average removal rate of 92%. The propagation and leakage of invertebrates occurred in the sand and BAC filters but more seriously in the latter. The average reproduction rate in the BAC filter was 268.8% with rotifers as the taxon that leaked the most. Invertebrate survival and reproduction were also observed in the chlorine-disinfected clean water reservoir with an average reproduction rate of 41.9%. Owing to differences in chlorine resistance, the reproduction ability of the dominant taxa was in the order nematodes>crustaceans>rotifers. The proportion of endogenous invertebrates gradually increased along the treatment process. The average proportion of endogenous invertebrates in the finished water was higher than 79.0%. Our findings suggested that waterworks should pay more attention to endogenous invertebrate growth.

关键词: Invertebrates     Drinking water     Seasonal variations     Treatment process    

Applying chemical sedimentation process in drinking water treatment plant to address the emergent arsenicspills in water sources

Pengfei LIN,Xiaojian ZHANG,Hongwei YANG,Yong LI,Chao CHEN

《环境科学与工程前沿(英文)》 2015年 第9卷 第1期   页码 50-57 doi: 10.1007/s11783-014-0733-2

摘要: Arsenic (As) spills occurred more frequently and sometimes polluted water sources in recent years in China. It is as urgent need to develop emergency treatment technologies to address the arsenic threat for large-scale water treatment plants. In response, we developed a chemical sedimentation technology to remove arsenic contaminants for water treatment plants. Bench-scale experiments were conducted to investigate the efficiency of arsenic removal and the influencing factors of the chemical sedimentation treatment process. The influencing factors included the choice and dosage of coagulants, the valence of arsenic and pH value of solution. The As(V) contaminants can be almost completely removed by ferric or alum coagulants. The As(III) contaminants are more recalcitrant to chemical sedimentation, 75% for ferric coagulant and 40% for alum coagulant. The quantitative results of arsenic removal load by different ferric or alum coagulants were presented to help determine the parameters for arsenic treatment technology. The dominant mechanism for arsenic removal is static combination, or adsorption of negative arsenic species onto positive ferric hydroxide or alum hydroxide flocs. The efficiency of this treatment technology has also been demonstrated by a real production test in one water treatment plant with arsenic-rich source water and one emergency response. This technology was verified to be quick to set-up, easy to operate and highly efficient even for high concentration of arsenic.

关键词: Arsenic spill     chemical sedimentation     coagulation     drinking water     emergency treatment    

Effects of humic acid on residual Al control in drinking water treatment plants with orthophosphate addition

Wendong WANG, Hua LI, Zhenzhen DING, Xiaochang WANG, Rui LIU

《环境科学与工程前沿(英文)》 2012年 第6卷 第4期   页码 470-476 doi: 10.1007/s11783-012-0422-y

摘要: This study aimed to investigate the effects of humic acid (HA) on residual Al control in drinking water facilities that used orthophosphate addition. The results showed that adding orthophosphate was an effective method for residual Al control for the raw water without HA. When orthophosphate was added at 1.0 min before the addition of poly aluminum chloride (PACl), the concentrations of soluble aluminum (Sol-Al) and total aluminum (Tot-Al) residue were 0.08 and 0.086 mg·L , respectively; both were reduced by 46% compared with the control experiment. The presence of HA would notably increase the residual Al concentration. For the raw water with 5 mg·L of HA, the concentrations of Sol-Al and Tot-Al increased from 0.136 and 0.174 mg·L to 0.172 and 0.272 mg·L , respectively. For water with a HA concentration above 5 mg·L , orthophosphate was ineffective in the control of residual Al, though there were still parts of orthophosphate were removed in coagulation. The amounts of Al removal were positively correlated with the solids freshly formed in coagulation. Similar to the raw water without HA, the best Al control was obtained with orthophosphate salt added at 1.0 min before PACl. HA concentrations in the raw water, solution pH, and the orthophosphate dosage suitable for residual Al control by orthophosphate precipitation were also investigated.

关键词: coagulation     drinking water     humic acid     orthophosphate     residual Al    

Treatment, residual chlorine and season as factors affecting variability of trihalomethanes in smalldrinking water systems

Roberta DYCK,Geneviève COOL,Manuel RODRIGUEZ,Rehan SADIQ

《环境科学与工程前沿(英文)》 2015年 第9卷 第1期   页码 171-179 doi: 10.1007/s11783-014-0750-1

摘要: Seasonal variability in source water can lead to challenges for drinking water providers related to operational optimization and process control in treatment facilities. The objective of this study is to investigate seasonal variability of water quality in municipal small water systems (<3000 residents) supplied by surface waters. Residual chlorine and trihalomethanes (THM) were measured over seven years (2003–2009). Comparisons are made within each system over time, as well as between systems according to the type of their treatment technologies. THM concentrations are generally higher in the summer and autumn. The seasonal variability was generally more pronounced in systems using chlorination plus additional treatment. Chloroform, total THM (TTHM) and residual chlorine concentrations were generally lower in systems using chlorination plus additional treatment. Conversely, brominated THM concentrations were higher in systems using additional treatment. Residual chlorine was highest in the winter and lowest in the spring and summer. Seasonal variations were most pronounced for residual chlorine in systems with additional treatment. There was generally poor correlation between THM concentrations and concentrations of residual chlorine. Further study with these data will be beneficial in finding determinants and indicators for both quantity and variability of disinfection byproducts and other water quality parameters.

关键词: drinking water     residual chlorine     seasonal variability     small municipal systems     treatment technologies     trihalomethanes    

Using loose nanofiltration membrane for lake water treatment: A pilot study

《环境科学与工程前沿(英文)》 2021年 第15卷 第4期 doi: 10.1007/s11783-020-1362-6

摘要:

• A pilot study was conducted for drinking water treatment using loose NF membranes.

关键词: Nanofiltration     Drinking water     Membrane fouling     Aluminum carryover     Chemical cleaning    

dissemination and removal of antibiotic resistant bacteria and antibiotic resistance genes in urban drinkingwater system: A review

Qiaowen Tan, Weiying Li, Junpeng Zhang, Wei Zhou, Jiping Chen, Yue Li, Jie Ma

《环境科学与工程前沿(英文)》 2019年 第13卷 第3期 doi: 10.1007/s11783-019-1120-9

摘要:

Reviewed the change of ARGs and ARB in full-scale urban drinking water systems.

Conventional processes are more promising than BAC process in ARGs removal.

Mechanisms of ARGs enrichment and spread in BAC filter and DWDSs are discussed.

Raise the need of future research on ARGs and ARB change in building plumbing systems.

关键词: Antibiotic resistant bacteria     Antibiotic resistance genes     Water source     Drinking water treatment plant     Drinking water distribution system     Urban drinking water system    

Biofiltration and disinfection codetermine the bacterial antibiotic resistome in drinking water: A review

Kun Wan, Wenfang Lin, Shuai Zhu, Shenghua Zhang, Xin Yu

《环境科学与工程前沿(英文)》 2020年 第14卷 第1期 doi: 10.1007/s11783-019-1189-1

摘要: Published data was used to analyze the fate of ARGs in water treatment. Biomass removal leads to the reduction in absolute abundance of ARGs. Mechanism that filter biofilm maintain ARB/ARGs was summarized. Potential BAR risks caused by biofiltration and chlorination were proposed. The bacterial antibiotic resistome (BAR) is one of the most serious contemporary medical challenges. The BAR problem in drinking water is receiving growing attention. In this study, we focused on the distribution, changes, and health risks of the BAR throughout the drinking water treatment system. We extracted the antibiotic resistance gene (ARG) data from recent publications and analyzed ARG profiles based on diversity, absolute abundance, and relative abundance. The absolute abundance of ARG was found to decrease with water treatment processes and was positively correlated with the abundance of 16S rRNA (r2 = 0.963, p<0.001), indicating that the reduction of ARG concentration was accompanied by decreasing biomass. Among treatment processes, biofiltration and chlorination were discovered to play important roles in shaping the bacterial antibiotic resistome. Chlorination exhibited positive effects in controlling the diversity of ARG, while biofiltration, especially granular activated carbon filtration, increased the diversity of ARG. Both biofiltration and chlorination altered the structure of the resistome by affecting relative ARG abundance. In addition, we analyzed the mechanism behind the impact of biofiltration and chlorination on the bacterial antibiotic resistome. By intercepting influent ARG-carrying bacteria, biofilters can enrich various ARGs and maintain ARGs in biofilm. Chlorination further selects bacteria co-resistant to chlorine and antibiotics. Finally, we proposed the BAR health risks caused by biofiltration and chlorination in water treatment. To reduce potential BAR risk in drinking water, membrane filtration technology and water boiling are recommended at the point of use.

关键词: Drinking water treatment     Antibiotic resistance gene     Biofiltration     Chlorination    

Development and application of innovative technologies for drinking water quality assurance in China

QU Jiuhui, YIN Chengqing, YANG Min, LIU Huijuan

《环境科学与工程前沿(英文)》 2007年 第1卷 第3期   页码 257-269 doi: 10.1007/s11783-007-0044-y

摘要: The continuously deteriorating quality of source water is threatening the safety of drinking water in China. Various efforts have been made to update water treatment processes to decrease the pollution problems of drinking water, such as protection of drinking water sources, enhancement of conventional treatment processes, and development of new or advanced treatment technologies. This paper reviews a variety of protection and remediation methods for drinking water sources, development and application of drinking water treatment technologies, new technologies for special pollutants removal from groundwater, and the latest research progress on water distribution systems in China. treatment plant improvement is the key to ensure the quality of drinking water. There have been many researches on innovative treatment technologies in China and they have been applied in quite a number of water treatment plants. These innovations include key technique development and combination of technologies in the scope of economic optimization. On the basis of water quality from the plant, the distribution system is also important. This paper describes the latest development in the above respects.

关键词: advanced treatment     economic optimization     Various     enhancement     improvement    

Hexavalent chromium in drinking water: Chemistry, challenges and future outlook on Sn(II)- and photocatalyst-basedtreatment

Haizhou Liu, Xuejun Yu

《环境科学与工程前沿(英文)》 2020年 第14卷 第5期 doi: 10.1007/s11783-020-1267-4

摘要: Abstract • Wide occurrence of Cr(VI) in US source drinking water. • A strong dependence of occurrence on groundwater sources. • Elucidate Redox and equilibrium chemistry of Cr(VI). • Sn(II)-based and TiO2-based reductive treatments hold extreme promise. • Key challenges include residual waste, Cr(VI) re-generation and socioeconomic drivers. Chromium (Cr) typically exists in either trivalent and hexavalent oxidation states in drinking water, i.e., Cr(III) and Cr(VI), with Cr(VI) of particular concern in recent years due to its high toxicity and new regulatory standards. This Account presented a critical analysis of the sources and occurrence of Cr(VI) in drinking water in the United States, analyzed the equilibrium chemistry of Cr(VI) species, summarized important redox reaction relevant to the fate of Cr(VI) in drinking water, and critically reviewed emerging Cr(VI) treatment technologies. There is a wide occurrence of Cr(VI) in US source drinking water, with a strong dependence on groundwater sources, mainly due to naturally weathering of chromium-containing aquifers. Challenges regarding traditional Cr(VI) treatment include chemical cost, generation of secondary waste and inadvertent re-generation of Cr(VI) after treatment. To overcome these challenges, reductive Cr(VI) treatment technologies based on the application of stannous tin or electron-releasing titanium dioxide photocatalyst hold extreme promise in the future. To moving forward in the right direction, three key questions need further exploration for the technology implementation, including effective management of residual waste, minimizing the risks of Cr(VI) re-occurrence downstream of drinking water treatment plant, and promote the socioeconomic drivers for Cr(VI) control in the future.

关键词: Chromium     Chemistry     Treatment     Future outlook    

Characteristics and removal mechanism of the precursors of N-chloro-2,2-dichloroacetamide in a drinkingwater treatment process at Taihu Lake

《环境科学与工程前沿(英文)》 2021年 第15卷 第5期 doi: 10.1007/s11783-020-1338-6

摘要:

• N-Cl-DCAM, an emerging N-DBP in drinking water was investigated.

关键词: N-chloro-2     2-dichloroacetamide     Liquid chromatography with tandem mass spectrometry     Precursors     Removal efficiency     Ozonation integrated with biological activated carbon    

PPCPs in a drinking water treatment plant in the Yangtze River Delta of China: Occurrence, removal and

Xinshu Jiang, Yingxi Qu, Liquan Liu, Yuan He, Wenchao Li, Jun Huang, Hongwei Yang, Gang Yu

《环境科学与工程前沿(英文)》 2019年 第13卷 第2期 doi: 10.1007/s11783-019-1109-4

摘要:

• 39 PPCPs were investigated at a DWTP using the Yangtze River as its water source.

• Grab and continuous sampling were conducted for the comparison of data consistency.

• Ketoprofen & carbamazepine can be risk management indicators because of the high RQ.

关键词: PPCPs     DWTP     Human health risk assessment    

标题 作者 时间 类型 操作

Nanofiltration for drinking water treatment: a review

期刊论文

Emergency drinking water treatment in source water pollution incident-technology and practice in China

Xiaojian ZHANG , Chao CHEN ,

期刊论文

What have we known so far about microplastics in drinking water treatment? A timely review

期刊论文

Comparative genotoxicity of water processed by three drinking water treatment plants with different watertreatment procedures

Ting Zhang, Heze Liu, Yiyuan Zhang, Wenjun Sun, Xiuwei Ao

期刊论文

Seasonal and treatment-process variations in invertebrates in drinking water treatment plants

Zhiling Wu, Xianchun Tang, Hongbin Chen

期刊论文

Applying chemical sedimentation process in drinking water treatment plant to address the emergent arsenicspills in water sources

Pengfei LIN,Xiaojian ZHANG,Hongwei YANG,Yong LI,Chao CHEN

期刊论文

Effects of humic acid on residual Al control in drinking water treatment plants with orthophosphate addition

Wendong WANG, Hua LI, Zhenzhen DING, Xiaochang WANG, Rui LIU

期刊论文

Treatment, residual chlorine and season as factors affecting variability of trihalomethanes in smalldrinking water systems

Roberta DYCK,Geneviève COOL,Manuel RODRIGUEZ,Rehan SADIQ

期刊论文

Using loose nanofiltration membrane for lake water treatment: A pilot study

期刊论文

dissemination and removal of antibiotic resistant bacteria and antibiotic resistance genes in urban drinkingwater system: A review

Qiaowen Tan, Weiying Li, Junpeng Zhang, Wei Zhou, Jiping Chen, Yue Li, Jie Ma

期刊论文

Biofiltration and disinfection codetermine the bacterial antibiotic resistome in drinking water: A review

Kun Wan, Wenfang Lin, Shuai Zhu, Shenghua Zhang, Xin Yu

期刊论文

Development and application of innovative technologies for drinking water quality assurance in China

QU Jiuhui, YIN Chengqing, YANG Min, LIU Huijuan

期刊论文

Hexavalent chromium in drinking water: Chemistry, challenges and future outlook on Sn(II)- and photocatalyst-basedtreatment

Haizhou Liu, Xuejun Yu

期刊论文

Characteristics and removal mechanism of the precursors of N-chloro-2,2-dichloroacetamide in a drinkingwater treatment process at Taihu Lake

期刊论文

PPCPs in a drinking water treatment plant in the Yangtze River Delta of China: Occurrence, removal and

Xinshu Jiang, Yingxi Qu, Liquan Liu, Yuan He, Wenchao Li, Jun Huang, Hongwei Yang, Gang Yu

期刊论文